Publication Highlights of CRC1242

Highlights 2nd funding period

2023

Dimer Coupling Energies of the Si(001) Surface

Christian Brand, Alfred Hucht, Giriraj Jnawali, Jonas D. Fortmann, Björn Sothmann, Hamid Mehdipour, Peter Kratzer, Ralf Schützhold and Michael Horn-von Hoegen (Projects A2, B2, B3, B7, C3)

Phys. Rev. Lett. 130, 126203 (2023)

DOI: 10.1103/PhysRevLett.130.126203

Large Orbital Moment of Two Coupled Spin-Half Co Ions in a Complex on Gold

Chao Li, Roberto Robles, Nicolas Lorente, Sanjoy Kr Mahatha, Sebastian Rohlf, Kai Rossnagel, Alessandro Barla, Boris V. Sorokin, Stefano Rusponi, Philippe Ohresser, Sara Realista, Paulo N. Martinho, Torben Jasper-Toennies, Alexander Weismann, Richard Berndt and Manuel Gruber (Project A8)

ACS Nano (in press)

DOI: 10.1021/acsnano.3c01595

Density-Dependence of Surface Transport in Tellurium-Enriched Nanograined Bulk Bi2Te3

Sepideh Izadi, Ahana Bhattacharya, Sarah Salloum, Jeong-Woo Han, Lauritz Schnatmann, Ulrike Wolff, Nicolas Perez, Georg Bendt, Inga Ennen, Andreas Hütten, Kornelius Nielsch, Stephan Schulz, Martin Mittendorff and Gabi Schierning (Project B9)

Small 19, 2204850 (2023)

DOI: 10.1002/smll.202204850

Hydration at Highly Crowded Interfaces

Christopher Penschke, John Thomas, Cord Bertram, Angelos Michaelides, Karina Morgenstern, Peter Saalfrank and Uwe Bovensiepen (Project B1)

Phys. Rev. Lett. 130, 106202 (2023)

DOI: 10.1103/PhysRevLett.130.106202

Temperature-Dependent Photoconductivity in Two-Dimensional MoS2 Transistors

Antonio Di Bartolomeo, Arun Kumar, O. Durante, A. Sessa, Enver Faella, Loredana Viscardi, K. Intonti, Filippo Giubileo, N. Martucciello, P. Romano, Stephan Sleziona and Marika Schleberger (Project C5)

Materials Today Nano 24, 100382 (2023)

DOI: 10.1016/j.mtnano.2023.100382

2022

 Structural Changes across Thermodynamic Maxima in Supercooled Liquid Tellurium: A Water-Like Scenario

Peihao Sun, Giulio Monaco, Peter Zalden, Klaus Sokolowski-Tinten, Jerzy Antonowicz, Ryszard Sobierajski, Yukio Kajihara, Alfred Q. R. Baron, Paul Fuoss, Andrew Chihpin Chuang, Jun-Sang Park, Jonathan Almer and J. B. Hastings (Project C1)

Proc. Natl. Acad. Sci. USA 119, e2202044119 (2022)

DOI: 10.1073/pnas.2202044119

Experimental Characterization Techniques for Plasmon-Assisted Chemistry

Emiliano Cortés, Roland Grzeschik, Stefan A. Maier and Sebastian Schlücker (Project A4)

Nat. Rev. Chem. 6, 259 (2022)

DOI: 10.1038/s41570-022-00368-8

 Electronic Energy Transport in Nanoscale Au/Fe Hetero-Structures in the Perspective of Ultrafast Lattice Dynamics

Maximilian Mattern, Alexander von Reppert, Steffen Peer Zeuschner, Jan-Etienne Pudell, Florian Kühne, Detlef Diesing, Marc Herzog and Matias Bargheer (Project B1)

Appl. Phys. Lett. 120, 092401 (2022)
 

Pushing the Limits in Real-Time Measurements of Quantum Dynamics

Eric Kleinherbers, Philipp Stegmann, Annika Kurzmann, Martin Paul Geller, Axel Lorke and Jürgen König
(Projects A1, A2)

Phys. Rev. Lett. 128, 087701 (2022)

DOI: 10.1103/PhysRevLett.128.087701

Spin Crossover in a Cobalt Complex on Ag(111)

Sven Johannsen, Sascha Ossinger, Jan Grunwald, Alexander Herman, Heiko Wende, Felix Tuczek, Manuel Gruber and Richard Berndt (Projects A5, A8)

Angew. Chem. Int. Ed. 61, e202115892 (2022)

DOI: 10.1002/anie.202115892

Mass Transport via In-Plane Nanopores in Graphene Oxide Membranes

Tobias Foller, Lukas Madauß, Dali Ji, Xiaojun Ren, K. Kanishka H. De Silva, Tiziana Musso, Masamichi Yoshimura, Henning Lebius, Abdenacer Benyagoub, Priyank V. Kumar, Marika Schleberger and Rakesh Joshi (Project C5)

Nano Lett. 22, 4941 (2022)

DOI: 10.1021/acs.nanolett.2c01615

The Role of Electrons During the Martensitic Phase Transformation in NiTi-Based Shape Memory Alloys

Alexander Kunzmann, Jan Frenzel, Ulrike Wolff, Jeong-Woo Han, Lars Giebeler, David Piorunek, Martin Mittendorff, Juliane Scheiter, Heiko Reith, Nicolas Perez, Kornelius Nielsch, Gunther Eggeler and Gabi Schierning (Project B9)

Materials Today Physics 100671 (2022)

DOI: 10.1016/j.mtphys.2022.100671

2021

Segregation-Enhanced Epitaxy of Borophene on Ir(111) by Thermal Decomposition of Borazine

Karim Omambac, Marin Petrović, Pantelis Bampoulis, Christian Brand, Marko A. Kriegel, Pascal Dreher, David Janoschka, Ulrich Hagemann, Nils Hartmann, Philipp Valerius, Thomas Michely, Frank Meyer zu Heringdorf and Michael Horn-von Hoegen
(Projects B4, B6)

ACS Nano 15, 7421 (2021)

DOI: 10.1021/acsnano.1c00819

Interface‐Dominated Topological Transport in Nanograined Bulk Bi2Te3

Sepideh Izadi, Jeong Woo Han, Sarah Salloum, Ulrike Wolff, Lauritz Schnatmann, Aswin Vijai Asaithambi, Sebastian Matschy, Heike Schlörb, Heiko Reith, Nicolas Perez, Kornelius Nielsch, Stephan Schulz, Martin Mittendorff and Gabi Schierning
(Project B9)

Small 2021, 2103281 (2021)

DOI: 10.1002/smll.202103281

Violation of Boltzmann Equipartition Theorem in Angular Phonon Phase Space Slows down Nanoscale Heat Transfer in Ultrathin Heterofilms

Anja Hanisch-Blicharski, Verena Tinnemann, Simone Wall, Fabian Thiemann, Thorben Groven, Jonas Darius Fortmann, Mohammad Tajik, Christian Brand, Bengt-Olaf Frost, Alexander von Hoegen and Michael Horn-von Hoegen
(Project B4)

Nano Lett. 21, 7145 (2021)

DOI: 10.1021/acs.nanolett.1c01665

Electron Waiting Times in a Strongly Interacting Quantum Dot: Interaction Effects and Higher-Order Tunneling Processes

Philipp Stegmann, Björn Sothmann, Jürgen König and Christian Flindt (Project A2)

Phys. Rev. Lett. 127, 096803 (2021)

DOI: 10.1103/PhysRevLett.127.096803

Competition Between Coulomb and van der Waals Interactions in Xe-Cs+ Aggregates on Cu(111) Surfaces

John Thomas, C. Bertram, János Daru, Jayita Patwari, I. Langguth, Ping Zhou, Dominik Marx, Karina Morgenstern and Uwe Bovensiepen (Project B1)

Phys. Rev. Lett. 127, 266802 (2021)

DOI: 10.1103/PhysRevLett.127.266802

 Non-Conventional Bell-Shaped Diffuse Scattering in Low-Energy Electron Diffraction from High-Quality Epitaxial 2D-Materials

Karim Omambac, Marko Kriegel, Christian Brand, B. Finke, Laurenz Kremeyer, H. Hattab, David Janoschka, Pascal Dreher, Frank Meyer zu Heringdorf, Davood Momeni Pakdehi, Klaus Pierz, H.W. Schumacher, Marin Petrović, Arie van Houselt, B. Poelsema, M.C. Tringides and Michael Horn-von Hoegen (Projects B4, B6)

Appl. Phys. Lett. 118, 241902 (2021)

2020

High-Frequency Gas Effusion through Nanopores in Suspended Graphene

Irek E. Rosłoń, Robin J. Dolleman, H. Licona, Martin Lee, Makars Šiškins, Henning Lebius, Lukas Madauß, Marika Schleberger, Farbod Alijani, Herre Sjoerd Jan van der Zant and Peter G. Steeneken
(Project C5)

Nat. Commun. 11, 6025 (2020)

DOI: 10.1038/s41467-020-19893-5

2D THz Optoelectronics 

Martin Mittendorff, Stephan Winnerl and Thomas E. Murphy
(Project B9)

Adv. Optical Mater. 9, 2001500 (2020)

DOI: 10.1002/adom.202001500

 

Local and Nonlocal Electron Dynamics of Au/Fe/MgO(001) Heterostructures Analyzed by Time-Resolved Two-Photon Photoemission Spectroscopy

Yasin Beyazit, J. Beckord, Ping Zhou, Jan-Philipp Meyburg, Florian Kühne, Detlef Diesing, Manuel Ligges and Uwe Bovensiepen (Project B1)

Phys. Rev. Lett. 125, 076803 (2020)

Highlights 1st funding period

2020

Ultrafast Vector Imaging of Plasmonic Skyrmion Dynamics with Deep Subwavelength Resolution

Timothy J. Davis, David Janoschka, Pascal Dreher, Bettina Frank, Frank Meyer zu Heringdorf and Harald Giessen
(Project B6)

Science 368, 6415 (2020)

DOI: 10.1126/science.aba6415

Ultrafast Terahertz Magnetometry 

Wentao Zhang, Pablo Maldonado, Zuanming Jin, Tom S. Seifert, Jacek Arabski, Guy Schmerber, Eric Beaurepaire, Mischa Bonn, Tobias Kampfrath, Peter M. Oppeneer and Dmitry Turchinovich
(Project B8)

Nat. Commun. 11, 4247 (2020)

DOI: 10.1038/s41467-020-17935-6

Dynamical Control over Terahertz Electromagnetic Interference Shielding with 2D Ti₃C₂Ty MXene by Ultrafast Optical Pulses

Guangjiang Li, Naaman Amer, Hassan A. Hafez, Shuohan Huang, Dmitry Turchinovich, Vadym N. Mochalin, Frank A. Hegmann and Lyubov V. Titova
(Project B8)

Nano Lett. 20, 636 (2020)

DOI: 10.1021/acs.nanolett.9b04404

2019

Phonon Pair Creation by Inflating Quantum Fluctuations in an Ion Trap

Matthias Wittemer, Frederick Hakelberg, Philip Kiefer, Jan-Philipp Schröder, Christian Fey, Ralf Schützhold, Ulrich Warring and Tobias Schaetz (Projects B3, B7)

Phys. Rev. Lett. 123, 180502 (2019)

DOI: 10.1103/PhysRevLett.123.180502

Femtosecond X-Ray Diffraction Reveals a Liquid-Liquid Phase Transition in Phase-Change Materials

Peter Zalden, Florian Quirin, Mathias Schumacher, Jan Siegel, Shuai Wei, Azize Koc, Matthieu Nicoul, Mariano Trigo, Pererik Andreasson, Henrik Enquist, Michael J. Shu, Tommaso Pardini, Matthieu Chollet, Diling Zhu, Henrik Lemke, Ider Ronneberger, Jörgen Larsson, Aaron M. Lindenberg, Henry E. Fischer, Stefan Hau-Riege, David A. Reis, Riccardo Mazzarello, Matthias Wuttig and Klaus Sokolowski-Tinten
(Project C1)

Science 364, 1062 (2019)

DOI: 10.1126/science.aaw1773

Porous Purple Glass - a Cobalt Imidazolate Glass with Accessible Porosity from a Meltable Cobalt Imidazolate Framework

Louis Frentzel-Beyme, Marvin Kloß, Roman Pallach, Soma Salamon, Henning Moldenhauer, Joachim Landers, Heiko Wende, Jörg Debus and Sebastian Henke
(Project A5)

J. Mater. Chem. A 7, 985 (2019)

DOI: 10.1039/c8ta08016j

Photon Noise Suppression by a Built-in Feedback Loop

Amran Al-Ashouri, Annika Kurzmann, Benjamin Merkel, Arne Ludwig, Andreas D. Wieck, Axel Lorke and Martin Paul Geller
(Project A1)

Nano Lett. 19, 135 (2019)

DOI: 10.1021/acs.nanolett.8b03486

Spectral Screening of the Energy of Hot Holes over a Particle Plasmon Resonance

Evangelina Pensa, Julian Gargiulo, Alberto Lauri, Sebastian Schlücker, Emiliano Cortés and Stefan A. Maier
(Project A4)

Nano Lett. 19, 1867 (2019)

DOI: 10.1021/acs.nanolett.8b04950

Temperature-Controlled Rotational Epitaxy of Graphene

Karim Omambac, Hichem Hattab, Christian Brand, Giriraj Jnawali, Alpha T. N’Diaye, Johann Coraux, Raoul van Gastel, Bene Poelsema, Thomas Michely, Frank Meyer zu Heringdorf and Michael Horn-von Hoegen
(Project B4)

Nano Lett. 19, 4594 (2019)

DOI: 10.1021/acs.nanolett.9b01565

Terahertz Nonlinear Optics of Graphene: From Saturable Absorption to High‐Harmonics Generation

Hassan A. Hafez, Sergey Kovalev, Klaas‐Jan Tielrooij, Mischa Bonn, Michael Gensch and Dmitry Turchinovich
(Project B8)

Adv. Optical Mater. 1900771 (2019) 

DOI: 10.1002/adom.201900771

Optical Detection of Single-Electron Tunneling into a Semiconductor Quantum Dot

A. Kurzmann, P. Stegmann, J. Kerski, R. Schott, A. Ludwig, A. D. Wieck, J. Koenig, A. Lorke, and M. Geller (Projects A1, A2)

Phys. Rev. Lett. 122, 247403 (2019)

Thermally Induced Crossover from 2D to 1D Behavior in an Array of Atomic Wires: Silicon Dangling-Bond Solitons in Si(553)-Au

Bernd Hafke, Christian Brand, Tobias Witte, Björn Sothmann, Michael Horn-von Hoegen and S. C. Erwin (Project C3)

Phys. Rev. Lett. 124, 016102 (2020)

DOI: 10.1103/PhysRevLett.124.016102

2018

Extremely Efficient Terahertz High-Harmonic Generation in Graphene by Hot Dirac Fermions

Hassan A. Eid Hafez, Sergey Kovalev, Jan-Christoph Deinert, Zoltán Mics, Bertram Green, Nilesh Awari, Min Chen, Semyon Germanskiy, Ulf Lehnert, Jochen Teichert, Zhe Wang, Klaas-Jan Tielrooij, Zhaoyang Liu, Zongping Chen, Akimitsu Narita, Klaus Müllen, Mischa Bonn, Michael Gensch and Dmitry Turchinovich
(Project B8)

Nature 561, 507 (2018)

DOI: 10.1038/s41586-018-0508-1

Observation of Dicke Cooperativity in Magnetic Interactions

Xinwei Li, Motoaki Bamba, Ning Yuan, Qi Zhang, Yage Zhao, Maolin Xiang, Kai Xu, Zuanming Jin, Wei Ren, Guohong Ma, Shixun Cao, Dmitry Turchinovich and Junichiro Kono
(Project B8)

Science 361, 794 (2018)

DOI: 10.1126/science.aat5162

Heterogeneous to Homogeneous Melting Transition Visualized with Ultrafast Electron Diffraction

M. Z. Mo, Z. Chen, R. K. Li, M. Dunning, B. B. L. Witte, J. K .Baldwin, L. B Fletcher, J. B. Kim, A. Ng, R. Redmer, A H Reid, P. Shekhar, X. Z. Shen, M. Shen, K. Sokolowski-Tinten, Y. Y. Tsui, Y Q Wang, Q. Zheng, X. J. Wang and S. H. Glenzer
(Project C1)

Science 360, 1451 (2018)

DOI: 10.1126/science.aar2058

Nonequilibrium Electron and Lattice Dynamics of Strongly Correlated Bi2Sr2CaCu2O8+δ Single Crystals

Tatiana Konstantinova, Jonathan D. Rameau, Alexander H. Reid, Omadillo Abdurazakov, Lijun Wu, Renkai Li, Xiaozhe Shen, Genda Gu, Yuan Huang, Laurenz Rettig, Isabella Avigo, Manuel Ligges, James K. Freericks, Alexander F. Kemper, Hermann A. Dürr, Uwe Bovensiepen, Peter D. Johnson, Xijie Wang and Yimei Zhu
(Project B1)

Science Adv. 4, 7427 (2018)

DOI: 10.1126/sciadv.aap7427

Delayed Onset of Nonthermal Melting in Single-Crystal Silicon Pumped with Hard X Rays

J. Robinson, T. Decker, S. Guillet, T. Pardini, J. Koglin, R. Hill, A. E. Gleason, B. Kozioziemski, S. Boutet, Klaus Sokolowski-Tinten, A. Aquila, P. Hamilton, R. Soufli, J. Alameda, M. Hayes and S. P. Hau-Riege (Project C1)

Phys. Rev. Lett. 120, 265701 (2018)

DOI: 10.1103/PhysRevLett.120.265701

Ultrafast Doublon Dynamics in Photoexcited 1T - TaS2

M. Ligges, Isabella Avigo, D. Golež, H.U.R. Strand, Y. Beyazit, K. Hanff, F. Diekmann, L. Stojchevska, M. Kalläne, P. Zhou, K. Rossnagel, M. Eckstein, P. Werner and U. Bovensiepen (Project B1)

Phys. Rev. Lett. 120, 166401 (2018)

DOI: 10.1103/PhysRevLett.120.166401

2017

Optically Excited Structural Transition in Atomic Wires on Surfaces at the Quantum Limit

Tim Frigge, Bernd Hafke, Tobias Witte, Boris Krenzer, Carla Streubühr, Abdul Samad Syed, Vesna Mikšić Trontl, Isabella Avigo, Ping Zhou, Manuel Ligges, Dietrich von der Linde, Uwe Bovensiepen, Michael Horn-von Hoegen, Stefan Wippermann, Andreas Lücke, Simone Sanna, Uwe Gerstmann and Wolf Gerp Schmidt
(Projects B1, C3)

Nature 544, 207 (2017)

DOI: 10.1038/nature21432

Revealing the Subfemtosecond Dynamics of Orbital Angular Momentum in Nanoplasmonic Vortices

G. Spektor, D. Kilban, A. K. Mahro, B. Frank, S. Ristok, L. Gal, P. Kahl, D. Podbiel, S. Mathias, H. Giessen, F.-J. Meyer zu Heringdorf, M. Orenstein and M. Aeschlimann
(Project B6)

Science 355, 1187 (2017)

DOI: 10.1126/science.aaj1699

Imaging the Nonlinear Plasmoemission Dynamics of Electrons from Strong Plasmonic Fields

Daniel Podbiel, Philip Kahl, Andreas Makris, Bettina Frank, Simon Sindermann, Timothy J. Davis, Harald Giessen, Michael Horn-von Hoegen and Frank Meyer zu Heringdorf
(Project B6)

Nano Lett. 17, 6569 (2017)

DOI: 10.1021/acs.nanolett.7b02235

Short-Range Surface Plasmonics: Localized Electron Emission Dynamics from a 60-nm Spot on an Atomically Flat Single-Crystalline Gold Surface

Bettina Frank, Philip Kahl, Daniel Podbiel, Grisha Spektor, Meir Orenstein, Liwei Fu, Thomas Weiss, Michael Horn-von Hoegen, Timothy J Davis, Frank Meyer zu Heringdorf and Harald Giessen
(Project B6)

Science Adv. 3, e1700721 (2017)

DOI: 10.1126/sciadv.1700721

Creating Nanoporous Graphene with Swift Heavy Ions

H. Vázquez, E. Harriet Åhlgren, Oliver Ochedowski, Aleksi A. Leino, Rasim Mirzayev, Roland Kozubek, Henning Lebius, Marko Karlušic, Milko Jakšic, Arkady V. Krasheninnikov, Jani Kotakoski, Marika Schleberger, Kai Nordlund and Flyura G. Djurabekova
(Project C5)

Carbon 114, 511 (2017)

DOI: 10.1016/j.carbon.2016.12.015

Interatomic Coulombic Decay: The Mechanism for Rapid Deexcitation of Hollow Atoms

Richard A. Wilhelm, Elisabeth Gruber, Janine Schwestka, Roland Kozubek, Teresa I. Madeira, José P. Marques, Jacek Kobus, Arkady V. Krasheninnikov, Marika Schleberger and Friedrich Aumayr (Project C5)

Phys. Rev. Lett. 119, 103401 (2017)

DOI: 10.1103/PhysRevLett.119.103401

2016

Ultrafast Electronic Response of Graphene to a Strong and Localized Electric Field

Elisabeth Gruber, Richard A. Wilhelm, Rémi Pétuya, Valerie Smejkal, Roland Kozubek, Anke Hierzenberger, Bernhard C. Bayer, Iñigo Aldazabal, Andrey K. Kazansky, Florian Libisch, Arkady V. Krasheninnikov, Marika Schleberger, Stefan Facsko, Andrei G. Borisov, Andrés Arnau and Friedrich Aumayr
(Project C5)

Nat. Commun. 7, 13948 (2016)

DOI: 10.1038/ncomms13948